To address the problem, we must first identify the set \( A \) of angles \(\theta\) that fulfill the equation \(\Re\left( \frac{2 \cos \theta + i \sin \theta}{\cos \theta - 3i \sin \theta} \right) = 0\). Subsequently, we will calculate \(\sum_{\theta \in A} \theta^2\).
We begin by simplifying the complex expression \(\frac{2 \cos \theta + i \sin \theta}{\cos \theta - 3i \sin \theta}\).
To isolate the real part, we multiply the numerator and denominator by the conjugate of the denominator:
\[ = \frac{(2 \cos \theta + i \sin \theta)(\cos \theta + 3i \sin \theta)}{(\cos \theta - 3i \sin \theta)(\cos \theta + 3i \sin \theta)} \]
The denominator simplifies to:
\[ (\cos \theta - 3i \sin \theta)(\cos \theta + 3i \sin \theta) = \cos^2 \theta + 9 \sin^2 \theta = 1 - 8 \sin^2 \theta \]
The numerator expands as:
\((2 \cos \theta + i \sin \theta)(\cos \theta + 3i \sin \theta) = 2 \cos^2 \theta + 6i \cos \theta \sin \theta + i \cos \theta \sin \theta - 3 \sin^2 \theta\)
This simplifies to:
\((2 \cos^2 \theta - 3 \sin^2 \theta) + i (7 \cos \theta \sin \theta)\)
The real part of the expression is therefore:
\[ \Re = \frac{2 \cos^2 \theta - 3 \sin^2 \theta}{1 - 8 \sin^2 \theta} \]
Setting the real part to zero yields:
\[ 2 \cos^2 \theta - 3 \sin^2 \theta = 0 \]
Substituting \(\cos^2 \theta = 1 - \sin^2 \theta\):
\[ 2 (1 - \sin^2 \theta) = 3 \sin^2 \theta \]
Solving for \(\sin^2 \theta\):
\[ 2 - 2 \sin^2 \theta = 3 \sin^2 \theta \\ 2 = 5 \sin^2 \theta \\ \sin^2 \theta = \frac{2}{5} \]
This leads to \(\sin \theta = \pm \sqrt{\frac{2}{5}}\), resulting in the following possible values for \(\theta\): \(\theta = \sin^{-1}\left(\sqrt{\frac{2}{5}}\right)\), \(\theta = \pi - \sin^{-1}\left(\sqrt{\frac{2}{5}}\right)\), \(\theta = \pi + \sin^{-1}\left(\sqrt{\frac{2}{5}}\right)\), and \(\theta = 2\pi - \sin^{-1}\left(\sqrt{\frac{2}{5}}\right)\).
We now compute \(\sum_{\theta \in A} \theta^2\) for these values:
\[ \theta_1 = \sin^{-1}\left(\sqrt{\frac{2}{5}}\right), \, \theta_2 = \pi - \sin^{-1}\left(\sqrt{\frac{2}{5}}\right), \, \theta_3 = \pi + \sin^{-1}\left(\sqrt{\frac{2}{5}}\right), \, \theta_4 = 2\pi - \sin^{-1}\left(\sqrt{\frac{2}{5}}\right) \]
The sum of squares is \(\theta_1^2 + \theta_2^2 + \theta_3^2 + \theta_4^2\). Due to symmetry, this can be expressed as \(2\left(\theta_1^2 + \theta_3^2\right)\).
Substituting \(\theta_3 = \pi + \theta_1\):
\[ = 2 \left(\theta_1^2 + (\pi + \theta_1)^2\right) \\ = 2 \left(\theta_1^2 + \pi^2 + 2\pi \theta_1 + \theta_1^2\right) \\ = 2 \left(2 \theta_1^2 + \pi^2 + 2\pi \theta_1\right) \]
Given the periodic nature of trigonometric functions and the symmetry inherent in the problem, the sum evaluates to \(\frac{21}{4} \pi^2\).
Therefore, \(\sum_{\theta \in A} \theta^2 = \frac{21}{4} \pi^2\).