Step 1: Plan:
The off-diagonal entries cancel in the sum, which makes this quick.
Step 2: Steps:
Cofactors of a 2 by 2 matrix: swap the diagonal, flip the signs of the other two entries. The $-\tan\theta$ entries become $+\tan\theta$, so adding the matrices cancels them.
The diagonal gives $2\sec\theta$ in each place. Equal to $4$ means $\sec\theta = 2$, and $\theta = 60^{\circ} = \frac{\pi}{3}$.
Check the other options: $\sec\frac{\pi}{12}\approx 1.035$, $\sec\frac{\pi}{6}\approx 1.155$, $\sec\frac{\pi}{4} \approx 1.414$, none is $2$.
Final Answer:
The value is $\theta = \frac{\pi}{3}$, option (C).
\[ \boxed{\frac{\pi}{3}} \]