Step 1: Set up the sixth roots.
We solve $x^6 = 64 = 2^6$. The six roots all have modulus $2$ and are equally spaced by $60^\circ$ around the circle of radius $2$.
Step 2: Write the roots.
They are $x_k = 2\big(\cos\frac{k\pi}{3} + i\sin\frac{k\pi}{3}\big)$ for $k = 0,1,2,3,4,5$.
Step 3: Compute their real parts.
The real parts are $2\cos\frac{k\pi}{3}$: for $k=0,1,2,3,4,5$ these are $2,\ 1,\ -1,\ -2,\ -1,\ 1$.
Step 4: Keep only negative real parts.
The roots with negative real part are at $k=2,3,4$: \[ -1 + i\sqrt{3},\quad -2,\quad -1 - i\sqrt{3}. \]
Step 5: Add them.
The imaginary parts $+\sqrt{3}$ and $-\sqrt{3}$ cancel, leaving the real sum $(-1) + (-2) + (-1) = -4$.
Step 6: State the result.
So the sum is $-4$, which is option (C).
\[ \boxed{-4} \]