According to the Boltzmann Equation $S = k_B \ln \Omega$, if a system is in a state of "Perfect Order" (a perfect crystal at $0\text{ K}$), the number of microstates $\Omega$ and the entropy $S$ are
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The Third Law of Thermodynamics states that the entropy of a perfect crystal at absolute zero is exactly zero.
This corresponds to a single microstate ($\Omega = 1$), representing zero randomness.